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WASHINGTON — When the United States sits down with Iran early next month for face-to-face talks, the Iranian nuclear program will be at the top of the American agenda, even though Iranian officials insist it is off the table, Secretary of State Hillary Rodham Clinton said Tuesday.

“Iran says it has a number of issues it wishes to discuss with us,” Mrs. Clinton told reporters. “But what we are concerned about is discussing with them the questions surrounding their nuclear program and ambitions.”

She said the meeting, to be held Oct. 1, would fulfill President Obama’s pledge to engage with Iran. But she insisted that the United States would not be drawn into a lengthy and fruitless diplomatic dance with Iran, as some analysts have warned.

“We have no illusions about the Iranian government,... >>>